Another thing that makes me think for N is the fact that rather than being uneasy with the fact of being an unconventional couple (even for us in France !) they are on the contrary display it quite proudly. Sounds quite N-esque to me. Or at least unbrided N.
Most the facts you posted are correct. My observations is that awkward smile is common on intellectuals. More down-to-earth poeple tend to either not smile at all or having a frank smile, whereas people who grew up in a more polished environnement, even sanguine non-submissives ones, tend to "fake smile" (mouth closed or semi open) often, as a form of politeness. Of course, A- can influence this (smiling for avoid bad consequences) as well as P trait (convenance) or being in the political field (appearing kind to potential voters). But all of this to say that it seems to me that they're too many factors, especially out of the NPA spectrum, behind the "awkward smile" to link it solely to A- trait. I think if you search for "macron sourire" you'll find some pictures of him with a starry-eyed smile, quite typical of a N type, even if not gingival I admit. Hyperactive gesture may also stem from many factors such as high temperament or( in the video) due to the fact that he does not speaks his native language. It is natural to help yourself with hand gestures when you speak a foreign language more than your native one. It may also come from being in the political field (attracting visual attention). You're right for the quite intense eye gaze indeed, it's an interesting element I somehow dismissed, but I've not seen any trace of vindictiveness behind.
It is true that NA/-/= can be fashion addicts too (By the way she did not buy most of the fashion she wore, it was in fact furnished by the brands for representation and she bring back most of the clothes after), but for Brigitte though I lack informations about her she's quite independant, continuing teaching even as a first lady. She's not ill at ease at all with poeple even with her husband gone. I saw a video long ago of Brigitte berating (in a N maneer) her husband. Not very characteristic of A= behavior. Maybe NA- indeed but NA=... Well that seems unlikely to me but as I said I lack information about her.
And as a female teacher, judging from my experience, it is not rare for them to care for younger men's stuff or clothing, adolescents or even adults, as if they were messy children sometimes. I've seen it from a large panel of female teachers especially those who have/had children themselves. And not only teachers by the way, simply many mothers with the N trait.
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