The death entries for 1893 records only a death of a Alexander at Sunderland but the age shown eliminates your Alexander. He possibly died other than England and Wales or even possibly lost at sea. There does not appear to be a freeBMD death entry for Charlotte. This maybe that she re married and had a new surname or the couple had emigrated - apart from being a scholar she does not seem to appear on the later census again suggesting that she moved abroad.
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